Spectromicroscopy of electronic phase separation in KxFe2−ySe2 superconductor

نویسندگان

  • M. Bendele
  • A. Barinov
  • B. Joseph
  • D. Innocenti
  • A. Iadecola
  • A. Bianconi
  • H. Takeya
  • Y. Mizuguchi
  • Y. Takano
  • T. Noji
  • T. Hatakeda
  • Y. Koike
  • M. Horio
  • A. Fujimori
  • D. Ootsuki
  • T. Mizokawa
  • N. L. Saini
چکیده

Structural phase separation in AxFe2-ySe2 system has been studied by different experimental techniques, however, it should be important to know how the electronic uniformity is influenced, on which length scale the electronic phases coexist, and what is their spatial distribution. Here, we have used novel scanning photoelectron microscopy (SPEM) to study the electronic phase separation in KxFe2-ySe2, providing a direct measurement of the topological spatial distribution of the different electronic phases. The SPEM results reveal a peculiar interconnected conducting filamentary phase that is embedded in the insulating texture. The filamentary structure with a particular topological geometry could be important for the high Tc superconductivity in the presence of a phase with a large magnetic moment in AxFe2-ySe2 materials.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Floating-zone growth of KxFe2-ySe2 single crystals

The discovery of superconductivity at temperatures above 30 K in KxFe2-ySe2 compounds has attracted considerable attention [1]. The crystal structure of KxFe2-ySe2 descends from the well-known ThCr2Si2 structure with vacancies at the Fe sites. It was soon found that magnetism and superconductivity coexist in AxFe2-ySe2 (A = K, Rb, and Cs) [2-3]. Even in single crystals which show full shielding...

متن کامل

Origin of Pressure-induced Superconducting Phase in KxFe2−ySe2 studied by Synchrotron X-ray Diffraction and Spectroscopy

Pressure dependence of the electronic and crystal structures of KxFe2-ySe2, which has pressure-induced two superconducting domes of SC I and SC II, was investigated by x-ray emission spectroscopy and diffraction. X-ray diffraction data show that compressibility along the c-axis changes around 12 GPa, where a new superconducting phase of SC II appears. This suggests a possible tetragonal to coll...

متن کامل

Formation mechanism of superconducting phase and its three-dimensional architecture in pseudo-single-crystal KxFe2â‹TMySe2

We report how the superconducting phase forms in pseudo-single-crystal KxFe2−ySe2. In situ scanning electron microscopy (SEM) observation reveals that, as an order-disorder transition occurs, on cooling, most of the high-temperature iron-vacancy-disordered phase gradually changes into the iron-vacancy-ordered phase, whereas a small quantity of the high-temperature phase retains its structure an...

متن کامل

Influence of microstructure on superconductivity in KxFe2−ySe2 and evidence for a new parent phase K2Fe7Se8

The search for new superconducting materials has been spurred on by the discovery of iron-based superconductors whose structure and composition is qualitatively different from the cuprates. The study of one such material, KxFe2-ySe2 with a critical temperature of 32 K, is made more difficult by the fact that it separates into two phases-a dominant antiferromagnetic insulating phase K2Fe4Se5, an...

متن کامل

( 0 6 z 6 2 ) and Lattice Distortion

We report structurally tuned superconductivity in KxFe2−ySe2−zSz (0 6 z 6 2) phase diagram. Superconducting Tc is suppressed as S is incorporated into the lattice, eventually vanishing at 80% of S. The magnetic and conductivity properties can be related to stoichiometry on poorly occupied Fe1 site and the local environment of nearly fully occupied Fe2 site. The decreasing Tc coincides with the ...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره 4  شماره 

صفحات  -

تاریخ انتشار 2014